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- W2979686876 abstract "Correlation of molecular structure and its magnetic property gives a better understanding toward the design of magnetic materials with long-range magnetic order. Here we report two new cobalt-based coordination polymers that exhibited coexistence of long-range ferromagnetic (FM) order and spin-glass (SG) transition at below Tc. Different orientation of magnetic moments, arrangements, and variation in connectivity with the ligands might be responsible for the SG transition. The SG transition was characterized by bifurcation of zero-field-cooled and field-cooled splitting at Tf ≈ 9.9 K (for both compounds) and AC susceptibility measurements. DC magnetization revealed the FM transition at high temperature, followed by a low-temperature SG transition. Moreover, the peculiarity found in low-temperature χ′′(T) can be attributed to the complex interplay between antiferromagnetic and ferromagnetic interactions and the coexistence of the long-range FM order and SG phase. Optical bandgap and temperature-dependent resistivity measurements showed that these compounds are semiconducting in nature." @default.
- W2979686876 created "2019-10-18" @default.
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- W2979686876 date "2019-10-07" @default.
- W2979686876 modified "2023-10-16" @default.
- W2979686876 title "Reentrant Spin-Glass Behavior in Cobalt(II) Based Coordination Polymers" @default.
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- W2979686876 doi "https://doi.org/10.1021/acs.cgd.9b00908" @default.
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