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- W2980451852 endingPage "121912" @default.
- W2980451852 startingPage "121912" @default.
- W2980451852 abstract "One of the greatest challenges of robust self-healing materials is the confliction between high chain mobility for self-healing and a stable structure for mechanical strength. Herein, dangling 2-ureido-4[1H]-pyrimidione (UPy)-functionalized side groups were introduced into the hard segments of thermoplastic polyurethane (TPU) elastomers, where embedded the dynamic disulfide bonds in the main chain. The strong quadruple H-bonding interaction between UPy side groups acts as supramolecular crosslinkers enabling the TPU elastomer to have improved mechanical properties (tensile strength up to 25 MPa and toughness ~100 MJ m−3), and simultaneously the plasticizer effect of dangling side chain endows it with efficient healing ability at elevated temperatures (80–100 °C) comparable to its linear analogues. This strategy shows great potential in designing robust self-healing TPU elastomer employing weak dynamic covalent bonds, with wide promising applications as wearable electronics, coatings and adhesives." @default.
- W2980451852 created "2019-10-25" @default.
- W2980451852 creator A5004823075 @default.
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- W2980451852 date "2019-11-01" @default.
- W2980451852 modified "2023-10-14" @default.
- W2980451852 title "Towards mechanical robust yet self-healing polyurethane elastomers via combination of dynamic main chain and dangling quadruple hydrogen bonds" @default.
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- W2980451852 doi "https://doi.org/10.1016/j.polymer.2019.121912" @default.
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