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- W2980582058 abstract "Mid-infrared (mid-IR) femtosecond pulse technologies have enabled mode-selective multi-quantum vibrational excitation and have opened a way to control molecular reactions at electronic ground states. However, attempts at realization of vibrational control in the condensed-phase systems have been hampered so far by poor excitation efficiency and fast intramolecular vibrational relaxation. Introduction of plasmonics to ultrafast quantum control may resolve these issues and open a new avenue toward controlled ground-state chemistry. What is important here is that interaction between mid-IR light and molecular vibration can be substantially enhanced via surface plasmon excitation, which has been used in surface-enhanced IR absorption spectroscopy [1]. Recently, surface plasmons have been applied to nonlinear IR spectroscopy, where nonlinear signals have been substantially enhanced [2–4]. Here we report on successful driving of molecular ground-state dissociation in the condensed-phase for the first time, by employing mid-IR chirp-pulsed plasmonic near-fields." @default.
- W2980582058 created "2019-10-25" @default.
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- W2980582058 date "2019-06-01" @default.
- W2980582058 modified "2023-09-30" @default.
- W2980582058 title "Vibrational Ladder-Climbing and Molecular Ground-State Dissociation Driven by Mid-Infrared Chirp-Pulsed Plasmonic Near-Fields" @default.
- W2980582058 doi "https://doi.org/10.1109/cleoe-eqec.2019.8873130" @default.
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