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• W2980915321 abstract "The growing demands for reproducible and clean sources of power has prompted the exploitation of novel materials for solar-energy conversion; in any case, the improvement of their conversion efficiency remains a big challenge. We report a mixed-dimensional heterostructure to synchronously enhance charge separation and light-absorption of the photoanodes via the introduction of two-dimensional reduced graphene oxide and zero-dimensional CuSbS2 quantum dots on one-dimensional TiO2 arrays. The experimental results show that the graphene sheets with a low Fermi level and a superior electron mobility accept photo-excited electrons from TiO2 and enable fast electron transportation; while the CuSbS2 quantum dots promote the visible light-absorption of the photoanode. The synergistic effects in this mixed-dimensional (1D-2D-0D) heterostructure photoanode induce a markedly raised photoconversion efficiency of 1.2% at 0.3 V and a photocurrent density of 5.5 mA cm-2 at 0.4 V. Furthermore, the photocurrent density of the mixed-dimensional heterostructure exceeds previously reported TiO2-based photoanodes in neutral media. The improved photoelectrochemical properties are attributed to the synergistic-effect-induced highly organized, mixed-dimensional architectures. It is expected that the mixed-dimensional heterostructure photoanode will be a potential candidate for applications in environmental remediation and energy fields." @default.
• W2980915321 created "2019-10-25" @default.
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• W2980915321 date "2019-01-01" @default.
• W2980915321 modified "2023-10-11" @default.
• W2980915321 title "TiO2/graphene/CuSbS2 mixed-dimensional array with high-performance photoelectrochemical properties" @default.
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• W2980915321 doi "https://doi.org/10.1039/c9ra07237c" @default.
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• W2980915321 hasPublicationYear "2019" @default.
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