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• W2980960051 abstract "CeF3 displays favorable scintillation properties, which have been utilized for decades in various solid-state systems. Its emission undergoes multi-component decays, which were interpreted by lattice defects and so-called intrinsic features herein. This study of the complex equilibria in connection with photophysical behavior of the cerium(III)-fluoride system in solution gave us the possibility to reveal the individual contribution of the [CeIIIFx(H2O)9−x]3−x species to the photoluminescence. Spectrophotometry and spectrofluorometry (also in time-resolved mode) were used, and combined with sophisticated evaluation methods regarding both the complex equilibria and the kinetics of the photoinduced processes. The individual photophysical parameters of the [CeIIIFx(H2O)9−x]3−x complexes were determined. For the kinetic evaluation, three methods of various simplifications were applied and compared. The results indicated that the rates of some excited-state equilibrium processes were comparable to those of the emission decay steps. Our results also contribute to the explanation of the multi-component emission decays in the CeF3-containing scintillators, due to the various coordination environments of Ce3+, which can be affected by the excitation leading to the dissociation of the metal-ligand bonds." @default.
• W2980960051 created "2019-10-25" @default.
• W2980960051 creator A5007171936 @default.
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• W2980960051 date "2019-10-15" @default.
• W2980960051 modified "2023-10-15" @default.
• W2980960051 title "Explanation for the Multi-Component Scintillation of Cerium Fluoride Through the Equilibrium and Photophysical Investigation of Cerium(III)-Fluoro Complexes" @default.
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• W2980960051 doi "https://doi.org/10.3390/nano9101462" @default.
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• W2980960051 hasPublicationYear "2019" @default.
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