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• W2980969063 endingPage "121466" @default.
• W2980969063 startingPage "121466" @default.
• W2980969063 abstract "Organic phosphorus is an important source of eutrophication. In this study, to understand the mechanism of organophosphorus photodegradation, humic acid-Fe3+ (HA-Fe3+) complexes were prepared as a sensitizer, and glyphosate (GP) was used as a substrate for photodegradation. The effects of the initial GP concentration, HA concentration, Fe3+ concentration and microbial factors on photodegradation were investigated. The initial concentrations of GP, HA and Fe3+ could significantly affect the degradation rate of GP. Phosphate is the main product of GP photodegradation. Based on the identification of the active species in the reaction process, t-butanol was found to have the most significant inhibitory effect on the degradation. The reaction rate after t-butanol treatment was reduced from 0.017 to 0.003. This confirmed that OH was the main oxidant in the system, which was also demonstrated by EPR spectroscopy. A possible mechanism of GP photodegradation sensitized by HA-Fe3+ complexes was revealed for the first time. The HA-Fe3+ complexes in the reaction system were photodegraded and oxidized to finally produce OH, which promotes GP photodegradation. This study facilitates understanding the phosphorus cycle in a water environment and provides a scientific basis for the restoration of eutrophic lakes." @default.
• W2980969063 created "2019-10-25" @default.
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• W2980969063 date "2020-02-01" @default.
• W2980969063 modified "2023-10-16" @default.
• W2980969063 title "The mechanism of aquatic photodegradation of organophosphorus sensitized by humic acid-Fe3+ complexes" @default.
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• W2980969063 doi "https://doi.org/10.1016/j.jhazmat.2019.121466" @default.
• W2980969063 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/31679891" @default.
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