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- W2980969587 abstract "Microporous polyimides have been extensively investigated for CO2 capture and separation applications. Here, the crosslinked structure and the polar CO2-philic trifluoromethyl group are introduced into the hyperbranched polyimides to construct the microporous polyimide networks for efficient CO2 capture. The HBPI-CL networks exhibit significant increased micropores (pore size less than 1 nm) surface area and volume ranging from 79 to 89 m2g-1 and 0.03–0.05 cm3 g−1. It is intriguingly found that the CF3TAPA-HBPI-CL have more abundant ultramicropores and exhibit higher CO2 uptake capacity and CO2/N2 selectivity (8.56 wt% and 33.3) than those of TAPA-HBPI-CL (7.47 wt% and 20.4) without the polar CO2-philic trifluoromethyl group at 273 K/1 bar. This work reveals that the introduction of polar CO2-philic trifluoromethyl group into crosslinked polyimides is an effective method to improve the CO2 adsorption capacity and selectivity of microporous polyimide, which can be also applied to other microporous polymers." @default.
- W2980969587 created "2019-10-25" @default.
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- W2980969587 date "2020-02-01" @default.
- W2980969587 modified "2023-10-12" @default.
- W2980969587 title "Crosslinked microporous polyimides with polar substituent group for efficient CO2 capture" @default.
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- W2980969587 doi "https://doi.org/10.1016/j.micromeso.2019.109809" @default.
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