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• W2981042165 abstract "In this work, we successfully prepared three different mesoporous NiO nanostructures with preferential (111) planes using three different solvents-water, a water-ethanol mixture, and a water-ethylene glycol mixture. The NiO nanosheets prepared from the water-ethylene glycol mixture and denoted as NiO-EG showed a nanosheet morphology thinner than 10 nm, whereas the water-ethanol and water samples were 30-40 nm and above 100 nm thick, respectively. The NiO-EG catalyst was found to exhibit a high catalyzing ability to activate peroxymonosulfate (PMS) for decoloring dyes, by which 94.4% of acid orange 7 (AO7) was degraded under the following reaction conditions: AO7 = 50 mg/L, catalyst = 0.2 g/L, PMS = 0.8 g/L, pH = 7, and 30 min reaction time. The dye degradation rate was investigated as a function of the catalyst dosage, pH, and dye concentration. According to quenching experiments, it was found that SO4•-, HO•, and O2•- were the dominant radicals for AO7 degradation, and oxygen vacancies played a significant role in the generation of radicals. High surface area, thin flaky structure, rich oxygen vacancies, fast charge transport, and low diffusion impedance all enhanced the catalytic activity of NiO-EG, which exhibited the highest degradation ability due to its abundant accessible active sites for both adsorption and catalysis." @default.
• W2981042165 created "2019-10-25" @default.
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• W2981042165 date "2019-10-17" @default.
• W2981042165 modified "2023-10-17" @default.
• W2981042165 title "Solvent Effect on the Solvothermal Synthesis of Mesoporous NiO Catalysts for Activation of Peroxymonosulfate to Degrade Organic Dyes" @default.
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• W2981042165 doi "https://doi.org/10.1021/acsomega.9b01883" @default.
• W2981042165 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/6822129" @default.
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• W2981042165 hasPublicationYear "2019" @default.
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