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- W2981109265 abstract "FeOCl Fenton-like catalyst has drawn much attention due to its high catalytic activity. Nevertheless, the potential application of FeOCl is significantly hindered by the sluggish reduction kinetics of Fe3+ to active Fe2+. Here, we report that the incorporation of Fe - O-Mo electron mediator into FeOCl via forming a FeOCl/MoS2 composite can facilitate the Fe2+ regeneration through the oxidation of Mo4+ to Mo6+, which boosts the hydroxyl radicals yields, thus leading to a significantly improved catalytic performance. The removal efficiency of methylene blue (MB, 50 mg L-1) achieves ∼100% within 2 min. with low dosage of FeOCl/MoS2 (0.2 g L-1) and H2O2 (0.6 mM). FeOCl/MoS2 not only has broad working pH range (∼3 - 9) and high salinity tolerance (100 mM), but also capable to degrade various organic pollutants. For practical application, the fabricated FeOCl/MoS2 membrane effectively degrades continuous MB flow. This study demonstrates that incorporating an electron mediator is an effective way to improve the catalytic performance of heterogeneous Fenton-like catalysts." @default.
- W2981109265 created "2019-10-25" @default.
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- W2981109265 date "2020-02-01" @default.
- W2981109265 modified "2023-10-16" @default.
- W2981109265 title "Improving the Fenton catalytic performance of FeOCl using an electron mediator" @default.
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- W2981109265 doi "https://doi.org/10.1016/j.jhazmat.2019.121494" @default.
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