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• W2981264826 abstract "Developing 3 D self-assembled nanoarchitectures with well-defined crystal structures is an effective strategy to enhance the electrochemical performances of electrode materials. (1 1 0)-oriented and bridged-nanoblocks self-assembled VS4 microspheres are controllably synthesized by a facile one-step hydrothermal method. The (1 1 0)-bridged structure sets up open pathways for Na+ diffusion among nanoblocks, and the (1 1 0)-oriented structure provides unobstructed pathways for Na+ diffusion in the nanoblocks, which collectively constructs multidimensional Na+ transfer channels in the VS4 microspheres, promoting the electrochemical kinetics. As an anode for Na-ion batteries (SIBs), this material exhibits pseudocapacitive Na+ storage and excellent rate capability, delivering high capacities of 339 and 270 mAh g-1 at rates of 0.1 and 2.0 A g-1 , respectively, with a capacity retention of 79 % in the voltage window of 0.5-3.0 V. In particular, the reversible capacity reaches 575 mAh g-1 after 300 cycles even at 1.0 A g-1 in the voltage window of 0.05-3.0 V, outperforming those of the ever-reported VS4 -based anode materials. This work presents an effective strategy to the exploration and design of high-performance anodes for SIBs." @default.
• W2981264826 created "2019-10-25" @default.
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• W2981264826 date "2019-11-18" @default.
• W2981264826 modified "2023-10-11" @default.
• W2981264826 title "Enhanced Kinetics over VS ₄ Microspheres with Multidimensional Na ⁺ Transfer Channels for High‐Rate Na‐Ion Battery Anodes" @default.
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• W2981264826 doi "https://doi.org/10.1002/cssc.201902130" @default.
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• W2981264826 hasPublicationYear "2019" @default.
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