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• W2981479872 abstract "Electronic absorption spectra of water cluster anions (H2O)n-, n ≤ 200, at T = 80 K are obtained by photodissociation spectroscopy and compared with simulations from literature and experimental data for bulk hydrated electrons. Two almost isoenergetic electron binding motifs are seen for cluster sizes 20 ≤ n ≤ 40, which are assigned to surface and partially embedded isomers. With increasing cluster size, the surface isomer becomes less populated, and for n ≥ 50, the partially embedded isomer prevails. The absorption shifts to the blue, reaching a plateau at n ≈ 100. In this size range, the absorption spectrum is similar to that of the bulk hydrated electron but is slightly red-shifted; spectral moment analysis indicates that these clusters are reasonable model systems for hydrated electrons near the liquid-vacuum interface." @default.
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• W2981479872 date "2019-10-25" @default.
• W2981479872 modified "2023-10-12" @default.
• W2981479872 title "Probing the Structural Evolution of the Hydrated Electron in Water Cluster Anions (H₂O)_<i>n</i>^–, <i>n</i> ≤ 200, by Electronic Absorption Spectroscopy" @default.
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• W2981479872 doi "https://doi.org/10.1021/jacs.9b10347" @default.
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