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- W2981567160 abstract "Transition-metal-based phosphides (TMPs) have been considered as attractive electrocatalysts for water splitting due to their earth-abundance and remarkable catalytic activity. As a representative type of precursors, metal-organic frameworks (MOFs) provide ideal plateaus for the design of nanostructured TMPs. In this work, the hierarchically structured iron phosphide nanobundles (FeP-500) were fabricated by one-step phosphorization of an iron-based MOF (MET(Fe)) precursor. The derived FeP-500 nanobundles were constructed by quasi-paralleled one-dimensional nanorods with uneven surface, which provided channels for electrolyte penetration, mass transport, and effective exposure of active sites during the water-splitting process. With the addition of conductive Super P, the obtained FeP-500-S exhibited a good electrocatalytic performance towards the hydrogen evolution reaction in alkaline electrolyte (1 mol L-1 KOH). Furthermore, to investigate the influence of secondary metal doping, a series of isoreticular MOF precursors and bimetallic TMPs were fabricated. The results indicated that the catalytic performance is structure dominated." @default.
- W2981567160 created "2019-11-01" @default.
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- W2981567160 date "2019-11-26" @default.
- W2981567160 modified "2023-10-16" @default.
- W2981567160 title "Nanobundles of Iron Phosphide Fabricated by Direct Phosphorization of Metal–Organic Frameworks as an Efficient Hydrogen‐Evolving Electrocatalyst" @default.
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- W2981567160 doi "https://doi.org/10.1002/chem.201904280" @default.
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