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• W2981863864 abstract "Nonequilibrium deposition is a remarkable method for the in situ growth of unique nanostructures and phases for the functionalization of thin films. We introduce a distinctive structure of a mixed-phase, composed of BiVO4 and β-Bi2O3, for photoelectrochemical water splitting. The mixed-phase is fabricated via nonequilibrium deposition by adjusted oxygen partial pressure. According to density functional theory calculations, we find that vanadium exsolution can be facilitated by introducing oxygen vacancies, enabling the fabrication of a nanostructured mixed-phase. These unique structures enhance charge migration by increasing the interfacial area and properly aligning the band offset between two crystalline phases. Consequently, the photocurrent density of the nanostructured mixed-phase thin films is about twice that of pristine BiVO4 thin films at 1.23 VRHE. Our work suggests that nonequilibrium deposition provides an innovative route for the structural engineering of photoelectrodes for the understanding of fundamental properties and improving the photocatalytic performance for solar water splitting." @default.
• W2981863864 created "2019-11-01" @default.
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• W2981863864 date "2019-10-21" @default.
• W2981863864 modified "2023-10-18" @default.
• W2981863864 title "In Situ Growth of Nanostructured BiVO₄–Bi₂O₃ Mixed-Phase via Nonequilibrium Deposition Involving Metal Exsolution for Enhanced Photoelectrochemical Water Splitting" @default.
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• W2981863864 doi "https://doi.org/10.1021/acsami.9b12916" @default.
• W2981863864 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/31631650" @default.
• W2981863864 hasPublicationYear "2019" @default.
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