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- W2982492495 abstract "A kinetic model describing chemical reactions on a crystal surface is introduced. The Boltzmann equations involve particles interacting with potentials generated by fixed crystal particles and interacting with a phonon gas describing the fluctuating part of the potentials. Chemical reactions between gas/physisorbed, chemisorbed and crystal species are taken into account. The phonons are assumed to be at equilibrium for the sake of simplicity. A modified kinetic entropy is introduced for the coupled system and the H theorem is established. Using a fluid scaling and the Chapman-Enskog asymptotic method, species fluid boundary conditions involving heterogeneous reactions are recovered at the surface." @default.
- W2982492495 created "2019-11-08" @default.
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- W2982492495 date "2019-01-01" @default.
- W2982492495 modified "2023-09-27" @default.
- W2982492495 title "A kinetic model of reactive crystal surfaces A Kinetic Model of Reactive Crystal Surfaces" @default.
- W2982492495 hasPublicationYear "2019" @default.
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