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- W2982546007 abstract "We have investigated adsorption-induced deformation in graphene oxide framework materials (GOFs) using neutron diffraction at sample pressures up to 140 bar. GOFs, made by the solvothermal reaction of graphite oxide and benzene-1,4-diboronic acid, are a suitable candidate for deformation studies due to their narrow (∼1 nm), monodispersed, slit-shaped pores whose width can be measured by diffraction techniques. We have observed, in situ, a monotonic expansion of the slit width with increasing pressure upon adsorption of xenon, methane, and hydrogen under supercritical conditions. The expansion of ∼4% observed for xenon at a pressure of 48 bar is the largest deformation yet reported for supercritical adsorption on a carbonaceous material. We find that the expansion of the three gases can be mapped onto a common curve based solely on their Lennard-Jones parameters, in a manner similar to a law of corresponding states." @default.
- W2982546007 created "2019-11-08" @default.
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- W2982546007 date "2019-10-28" @default.
- W2982546007 modified "2023-09-29" @default.
- W2982546007 title "Adsorption-Induced Expansion of Graphene Oxide Frameworks: Observation by in Situ Neutron Diffraction" @default.
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- W2982546007 doi "https://doi.org/10.1021/acsomega.9b02589" @default.
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