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• W2982558465 startingPage "9336" @default.
• W2982558465 abstract "Super resolution microscopy (SRM) brings the advantages of optical microscopy to the imaging of nanostructured soft matter, and in colloidal microgels, promises to quantify variations of crosslink densities at unprecedented length scales. However, the distribution of all crosslinks does not coincide with that of dye-tagged crosslinks, and density quantification in SRM is not guaranteed due to over/under-counting dye molecules. Here we demonstrate that SRM images of microgels encode reaction rate constants of functional cross linkers, which hold the key to correlating these distributions. Combined with evolution of microgel particle radii, the functional cross linker distributions predict consumption versus time with high fidelity. Using a Bayesian regression approach, we extract reaction rate constants for homo and cross propagation of the functional crosslinker, which should be widely useful for predicting spatial variations in crosslink density of gels." @default.
• W2982558465 created "2019-11-08" @default.
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• W2982558465 date "2019-01-01" @default.
• W2982558465 modified "2023-10-13" @default.
• W2982558465 title "Quantification of functional crosslinker reaction kinetics<i>via</i>super-resolution microscopy of swollen microgels" @default.
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• W2982558465 doi "https://doi.org/10.1039/c9sm01618j" @default.
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• W2982558465 hasPublicationYear "2019" @default.
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