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- W2982652014 abstract "Organic aerosol is the largest fraction of the atmospheric nonrefractory aerosol mass and has a significant impact on climate, visibility, and human health. A significant portion of organic aerosol is secondary organic aerosol (SOA), which forms when volatile organic compounds (VOCs) are oxidized and the reaction products partition to the particle phase. SOA formation and aging have been described using semivolatile partitioning theory, and a typical assumption invoked is that gas-particle partitioning rapidly reaches equilibrium. However, several studies have called into question whether traditional equilibrium assumptions are valid, either due to particle-phase diffusion limitations, particle-phase reactions, or liquid/liquid phase separation and immiscibility of organic phases. Here, we investigate the ability of equilibrium partitioning to describe laboratory SOA formation experiments using SOA mass and yield as the evaluation metric. We conduct two types of experiments: (1) co-condensation experiment..." @default.
- W2982652014 created "2019-11-08" @default.
- W2982652014 creator A5012681365 @default.
- W2982652014 creator A5026616029 @default.
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- W2982652014 creator A5057022426 @default.
- W2982652014 creator A5074206807 @default.
- W2982652014 date "2019-10-28" @default.
- W2982652014 modified "2023-09-29" @default.
- W2982652014 title "Photochemical Aging Alters Secondary Organic Aerosol Partitioning Behavior" @default.
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