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- W2982665652 abstract "In this work, we used solvent vapor annealing as a route toward controlled cluster growth of a nitrogen-substituted terrylene molecule (7,8,15,16-tetrazaterrylene or TAT) to probe the underlying molecular packing behind the exciton band curvature (EBC) inversion leading to a so-called HJ aggregates. Using a suite of photoluminescence (PL) imaging tools, we show that the EBC—as signaled by PL spectral signatures—are correlated with distinct polarization and defocused emission patterns suggestive of a high degree of chromophore alignment. Selected area electron diffraction showed that the small aggregates adopt nominally the same crystal packing structure as the extended crystals though with a different plane orientation ([010] vs [011]) with respect to the surface normal. These findings demonstrate experimentally that the EBC inversion is not due to a crystal polymorphism but, rather subtle differences in molecular registration that profoundly impacts interchromophore coupling." @default.
- W2982665652 created "2019-11-08" @default.
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- W2982665652 date "2019-10-28" @default.
- W2982665652 modified "2023-10-12" @default.
- W2982665652 title "Probing the Evolution of Molecular Packing Underlying HJ-Aggregate Transition in Organic Semiconductors Using Solvent Vapor Annealing" @default.
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- W2982665652 doi "https://doi.org/10.1021/acs.jpcc.9b06814" @default.
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