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- W2982862918 abstract "Transition metal catalyzed ethylene copolymerization with polar monomers is a highly challenging reaction. After decades of research, the scope of suitable comonomer substrates has expanded from special to fundamental polar monomers and, recently, to 1,1-disubstituted ethylenes. Described in this contribution is a direct and tandem strategy to realize ethylene copolymerization with various 1,2-disubstituted ethylenes. The direct route is sensitive to sterics of both the comonomers and the catalyst. In the tandem route, ruthenium-catalyzed ethenolysis can convert 1,2-disubstituted ethylenes into terminal olefins, which can be subsequently copolymerized with ethylene to afford polar functionalized polyolefins. The one-pot, two-step tandem route is highly versatile and efficient in dealing with challenging substrates. This work is a step forward in terms of expanding the substrate scope for transition metal catalyzed ethylene copolymerization with polar-functionalized comonomers." @default.
- W2982862918 created "2019-11-22" @default.
- W2982862918 creator A5012718640 @default.
- W2982862918 creator A5035551783 @default.
- W2982862918 date "2019-12-12" @default.
- W2982862918 modified "2023-09-26" @default.
- W2982862918 title "Direct and Tandem Routes for the Copolymerization of Ethylene with Polar Functionalized Internal Olefins" @default.
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- W2982862918 doi "https://doi.org/10.1002/anie.201913088" @default.
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