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- W2983175537 abstract "The cycloaddition of epoxides and carbon dioxide represents a straightforward and atom-efficient method for synthesis of cyclic carbonates and utilization of CO2. So far, homogeneous metal complexes have been mainly applied for such transformations. Here, we describe the synthesis of novel heterogeneous Zn-based catalysts, which were conveniently prepared by pyrolysis of an active-carbon-supported phenanthroline-ligated Zn(OAc)2 complex. Detail structural characterizations proved the existence of single zinc sites in the active material. Compared to a Zn-based nanoparticle (Zn-NP) catalyst, the resulting single metal atom catalyst (SAC) displayed improved activity and stability for the cycloaddition of epoxides. By applying the optimal catalyst, a variety of carbonates were successfully obtained in high yields with good functional group tolerance." @default.
- W2983175537 created "2019-11-22" @default.
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- W2983175537 date "2019-11-01" @default.
- W2983175537 modified "2023-10-13" @default.
- W2983175537 title "Zinc single atoms on N-doped carbon: An efficient and stable catalyst for CO2 fixation and conversion" @default.
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- W2983175537 doi "https://doi.org/10.1016/s1872-2067(19)63316-4" @default.
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