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- W2983646788 abstract "主要组的交换离子的 ZSM-5 上的 N2O 的吸附和解吸附作用用规划温度的解吸附作用(TPD ) 和密度被学习功能的理论(DFT ) 计算。TPD 实验被执行在 metal-ion-exchanged ZSM-5s 上决定相应于 N2O 解吸附作用山峰的最大的集体紧张和 N2O 的吸附能力的使放出的温度 Tmax。结果显示 Tmax 跟随了 Ba2+ 的一个序列 >Ca2+>Cs+>K+>Na+> 主要组的金属阳离子上的吸附的 N2O 的数量跟随了的 Mg2+and Ba2+ 的一个序列 >Mg2+>Ca2+>Na+>K+>Cs+ 。DFT 计算被执行获得吸附精力(伊兹) ,它代表在 N2O 的金属阳离子和 N 结束或 O 结束之间的相互作用的力量。计算结果证明 N2O 分子的 N 结束有利地在交换离子的 ZSM-5 上被吸附,除了 Cs-ZSM-5。为碱金属阳离子,阳离子上的 N2O 的伊兹跟随了是对 Tmax 的一样的顺序:Cs+>K+>Na+ 。计算、试验性的结果一致地证明碱地球的金属阳离子的吸附表演比碱金属阳离子的那些好。" @default.
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- W2983646788 date "2011-01-01" @default.
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- W2983646788 title "Experimental and density functional theory study of the adsorption of N_2O on ion-exchanged ZSM-5: Part II. The adsorption of N_2O on main-group ion-exchanged ZSM-5" @default.
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