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• W2984162712 endingPage "15863" @default.
• W2984162712 startingPage "15853" @default.
• W2984162712 abstract "A series of neoteric 2-picolinate (pic)-decorated iron–lanthanide (Ln)-embedded germanotungstates (GTs), [LnIII(H2O)8]2H2[Fe4(H2O)4v(pic)4Ge2W20O72]·34 H2O [Ln = La (1), Ce (2), Nd (3), Sm (4), Gd (5), Tb (6), Dy (7), Er (8), Tm (9)] and [Eu(H2O)8]2H2[Fe4(H2O)4(pic)4Ge2W20O72]·36H2O (10; Hpic = picolinic acid), were hydrothermally prepared. The polyoxoanions of 1–10 possess a quadri-FeIII-inserted [Fe4(H2O)4(pic)4Ge2W20O72]8– subunit with bisupporting [Ln(H2O)8]3+ cations. The quadri-FeIII-inserted [Fe4(H2O)4 (pic)4Ge2W20O72]8– subunit can be described as a particular S-shaped [Ge2W20O72]16– segment functionalized by four [Fe(H2O)(pic)]2+ cations. It should be pointed out that the carboxyl O and pyridine N atoms on pic ligands simultaneously coordinate with Fe3+ cations in a five-membered heterocyclic mode, which can enhance the stability of the structures. Moreover, fluorescent measurements of 3, 4, 6, and 10 were made, manifesting that fluorescent emissions primarily stem from Ln3+ ions. With regard to 10, energy transfer (ET) from GT and pic groups to Eu3+ centers was intensively studied. In addition, the magnetic susceptibility properties of 7 and 10 were studied." @default.
• W2984162712 created "2019-11-22" @default.
• W2984162712 creator A5024924271 @default.
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• W2984162712 date "2019-11-14" @default.
• W2984162712 modified "2023-10-16" @default.
• W2984162712 title "2-Picolinate-Decorated Iron–Lanthanide Heterometallic Germanotungstates Including an S-Shaped [Ge₂W₂₀O₇₂]^16– Segment" @default.
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• W2984162712 doi "https://doi.org/10.1021/acs.inorgchem.9b02273" @default.
• W2984162712 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/31725268" @default.
• W2984162712 hasPublicationYear "2019" @default.
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