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- W2984776462 endingPage "45125" @default.
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- W2984776462 abstract "Metal-organic frameworks (MOFs) are powerful toolkits to directly correlate structure-function relationships due to their well-defined structures. In this work, 5,15-di(3,4,5-trihydroxyphenyl)porphyrin (DTPP) and 5,10,15,20-tetra(3,4,5-trihydroxyphenyl)porphyrin (TTPP) are reacted with zirconium ions to afford two MOFs (Zr-DTPP and Zr-TTPP) with acid and base tolerance in the pH range of 1.0-14.0. Powder X-ray diffraction investigation combined with Rietveld refinement reveals the J-aggregated porphyrin building blocks confined by benzene-1,2,3-trisolate-zirconium chains in the newly prepared Zr-DTPP. Electron spin-resonance, singlet-oxygen determination, and sulfides oxidation experiments demonstrate a much better singlet-oxygen evolution of J-aggregated Zr-DTPP than that of unaggregated Zr-TTPP reported previously, in good contrast to the weaker photocatalytic capability disclosed for DTPP than that for TTPP in solution, consummating the theory of photosensitizer J-aggregation in boosting heterogeneous photoinduced singlet-oxygen generation." @default.
- W2984776462 created "2019-11-22" @default.
- W2984776462 creator A5015991051 @default.
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- W2984776462 creator A5088303205 @default.
- W2984776462 date "2019-11-12" @default.
- W2984776462 modified "2023-10-15" @default.
- W2984776462 title "Elucidating J-Aggregation Effect in Boosting Singlet-Oxygen Evolution Using Zirconium–Porphyrin Frameworks: A Comprehensive Structural, Catalytic, and Spectroscopic Study" @default.
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- W2984776462 doi "https://doi.org/10.1021/acsami.9b17569" @default.
- W2984776462 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/31713412" @default.
- W2984776462 hasPublicationYear "2019" @default.
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