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- W2985364963 abstract "This contribution addresses the experimental observation and theoretical interpretation of environment-induced decoherence of molecular Schrodinger cat states, as observed for dihalogen molecules embedded in a cryogenic rare gas environment. We specifically address a three-pulse experiment performed on an (mathrm {I_2})-krypton system, involving the coherent creation, by two distinct optical pulses, of a vibrational Schrodinger cat state and its observation through a third pulse which induces a Raman scattering signal that reports on the time-evolving coherence. Full quantum-mechanical simulations of the combined molecule-plus-environment system under the influence of the external fields are reported, making use of advanced wave packet propagation techniques. As a key quantity, a time-evolving subsystem coherence matrix is characterized, and its evolution as a function of the state preparation is discussed. In line with the experiment, it is found that long-lived coherences can be observed, even though the system-bath coupling is comparatively strong. The system–environment interactions fall into a non-Markovian regime and are determined by a few specific environmental modes that strongly interact with the chromophore. A perspective is given on general implications of these observations for molecular systems embedded in a matrix or solvent environment." @default.
- W2985364963 created "2019-11-22" @default.
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- W2985364963 date "2019-01-01" @default.
- W2985364963 modified "2023-09-25" @default.
- W2985364963 title "Creation and Detection of Molecular Schrödinger Cat States: Iodine in Cryogenic Krypton Observed via Four-Wave-Mixing Optics" @default.
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- W2985364963 doi "https://doi.org/10.1007/978-3-030-31146-9_7" @default.
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