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• W2988467698 abstract "The synthesis and structure of atomically precise Au130-x Agx (average x=98) alloy nanoclusters protected by 55 ligands of 4-tert-butylbenzenethiolate are reported. This large alloy structure has a decahedral M54 (M=Au/Ag) core. The Au atoms are localized in the truncated Marks decahedron. In the core, a drum of Ag-rich sites is found, which is enclosed by a Marks decahedral cage of Au-rich sites. The surface is exclusively Ag-SR; X-ray absorption fine structure analysis supports the absence of Au-S bonds. The optical absorption spectrum shows a strong peak at 523 nm, seemingly a plasmon peak, but fs spectroscopic analysis indicates its non-plasmon nature. The non-metallicity of the Au130-x Agx nanocluster has set up a benchmark to study the transition to metallic state in the size evolution of bimetallic nanoclusters. The localized Au/Ag binary architecture in such a large alloy nanocluster provides atomic-level insights into the Au-Ag bonds in bimetallic nanoclusters." @default.
• W2988467698 created "2019-11-22" @default.
• W2988467698 creator A5005780047 @default.
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• W2988467698 date "2019-11-08" @default.
• W2988467698 modified "2023-09-29" @default.
• W2988467698 title "Au _{130− <i>x</i>} Ag _<i>x</i> Nanoclusters with Non‐Metallicity: A Drum of Silver‐Rich Sites Enclosed in a Marks‐Decahedral Cage of Gold‐Rich Sites" @default.
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• W2988467698 doi "https://doi.org/10.1002/anie.201908694" @default.
• W2988467698 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/31702861" @default.
• W2988467698 hasPublicationYear "2019" @default.
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