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- W2988848408 abstract "Abstract Gaseous carbon dioxide (CO2) was converted into few-layered graphene sheets grafted by carbon nanofibers (G-CNFs) at the atmospheric pressure. The synthesis was performed in a one-pot route by the thermal Mg-aided reduction of CO2 in the presence of nickel nanoparticles that have a crucial role in the growth of carbon nanofibers. The produced G-CNF was bifunctionally applied as a cathode supporter for elemental sulfur and a thin interlayer for the separator in the Li–S battery. The graphene layers exfoliated by the carbon nanofibers enabled the formation of semi-freestanding membrane through sonication in a surfactant solution. They were attached on the separator to be used as a several micron-thick interlayer. The G-CNF employed as both cathode and interlayer materials enhanced the charge-discharge capacity and stability due to its low electrical resistivity and its role as a barrier to the polysulfides shuttle. As a result, a high capacity of 820 mAhg−1 and 640 mA h g−1 after 100 and 500 cycles were acquired at 0.5 C, respectively. The results suggest not only the facile one-step conversion of atmospheric CO2 to the exfoliated graphene grafted by carbon nanofibers, but also its outstanding electrochemical performance in the Li–S battery." @default.
- W2988848408 created "2019-11-22" @default.
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- W2988848408 date "2020-01-01" @default.
- W2988848408 modified "2023-09-29" @default.
- W2988848408 title "One-pot conversion of carbon dioxide to CNT-grafted graphene bifunctional for sulfur cathode and thin interlayer of Li–S battery" @default.
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- W2988848408 doi "https://doi.org/10.1016/j.electacta.2019.135264" @default.
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