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- W2989136117 abstract "Before the large scale useof renewable energy sources can be implemented in our society,the storage of electrical energy needs to be tackled. Storage the energy ashydrogen via the reduction of protons is a good option. In order to form aclosed electrochemical cycle an oxidation reaction need to be used. The wateroxidation reaction is a good candidate as second reaction. When the energy isreleased, the oxygen reduction reaction is used to reduce the oxygen producedin the water oxidation reaction.This thesis focusses on heterogenized water oxidation and oxygen reductioncatalysts. Water oxidation occurs under highly oxidizing potentials. Thiscauses many molecular catalysts to degrade. In this thesis an example is givenof two pyridyl-triazolylidene iridium precatalysts which have different ratesof activation and deposition formation under reactive conditions.A copper-based catalyst has two different activation processes, an oxidativeand a reductive pathway, which stress the importance of choosing the rightreaction conditions before the start of catalysis.A copper complex with 1,10-phenanthroline ligands only forms an active oxygenreduction catalyst when one 1,10-phenanthroline ligand is coordinated to thecopper ion. By immobilizing the 1,10-phenanthroline ligand on the electrode, anactive heterogenized catalyst is formed." @default.
- W2989136117 created "2019-11-22" @default.
- W2989136117 creator A5052489093 @default.
- W2989136117 date "2019-10-10" @default.
- W2989136117 modified "2023-09-27" @default.
- W2989136117 title "Heterogenized molecular (pre)catalysts for water oxidation and oxygen reduction" @default.
- W2989136117 hasPublicationYear "2019" @default.
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