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- W2989357885 abstract "Based on (i) the low liquidus temperature of Si–Cu systems, (ii) low solubility of Cu in solid Si, and (iii) a strong affinity of Zr to B for the enhanced boride formation, a novel method to remove B from Si using Zr as a trapping agent via a Si–Cu solvent was developed in this study. B-bearing polygonal ZrBx precipitations found at the bottom of test samples were confirmed as ZrB2 by electron probe microanalysis. Thermodynamic analysis revealed that the solubility products of ZrB2 in a Si–Cu melt were 2.50 × 10–12 (1258 K, Si-57.0 atom % Cu) and 4.11 × 10–12 (1345 K, Si-50.0 atom % Cu). Finally, the compositions of Si–Cu alloys that can form stable ZrB2 particles were estimated by calculating the solubility products of ZrB2 and the equilibrium contents between B and Zr at different corresponding liquidus temperatures. The proposed method provides the potential for B removal via Si–Cu solvent refinement to realize the large-scale production of solar-grade silicon, thereby overcoming the key limitation to the sustainable utilization of solar energy." @default.
- W2989357885 created "2019-11-22" @default.
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- W2989357885 date "2019-11-07" @default.
- W2989357885 modified "2023-10-18" @default.
- W2989357885 title "Formation Mechanism of ZrB<sub>2</sub> in a Si–Cu Melt and Its Potential Application for Refining Si and Recycling Si Waste" @default.
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- W2989357885 doi "https://doi.org/10.1021/acssuschemeng.9b05986" @default.
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