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- W2989562014 abstract "Lithium-sulfur (Li–S) batteries have attracted increasing attention as one of the most promising candidates for next-generation energy storage systems. However, the shuttle effect of soluble intermediates, lithium polysulfides, results in a loss of active materials and sluggish redox kinetics, hampering the cyclability and rate capability of Li–S batteries. Here, we apply the commercial polypropylene separators modified with a 3D Ti3C2Tx aerogel to resolve the issues in Li–S batteries. This special structure of the Ti3C2Tx aerogel not only effectively avoids the restacking phenomenon of 2D Ti3C2Tx materials to expose more active surface and anchor lithium polysulfides but also increases the reaction kinetics of high-order lithium polysulfides to low-order lithium polysulfides, due to the high conductivity of Ti3C2Tx surfaces. Due to the high specific surface area and the 3D structure, the Li–S batteries with 3D Ti3C2Tx aerogel-functionalized separators exhibit superior performances, including a high discharge capacity of 1487 mAh g−1 at 0.1 C, a long cycling stability, and a low decay rate of 0.037% per cycle at 1 C for 1500 cycles." @default.
- W2989562014 created "2019-12-05" @default.
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- W2989562014 date "2020-03-01" @default.
- W2989562014 modified "2023-10-15" @default.
- W2989562014 title "3D Ti3C2Tx aerogel-modified separators for high-performance Li–S batteries" @default.
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- W2989562014 doi "https://doi.org/10.1016/j.jallcom.2019.153155" @default.
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