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• W2989689433 abstract "The electrochemical properties of carbon and reduced graphene-coated Na4Ni3(PO4)2P2O7 materials have been evaluated as high-voltage positive electrodes for sodium-ion batteries. Na4Ni3(PO4)2P2O7 exhibits the highest Ni3+/Ni2+ redox potential of 4.8 V vs. Na+/Na with a theoretical capacity of 127 mAh g−1. Here, we report on the synthesis and characterizations of Na4Ni3(PO4)2P2O7-reduced graphene oxide and Na4Ni3(PO4)2P2O7-carbon composites. The high-voltage dimethyl carbonate–based electrolyte has been chosen to explore the electrochemical properties of Na4Ni3(PO4)2P2O7 as a cathode. Carbon-coated Na4Ni3(PO4)2P2O7 composite electrode delivers a stable discharge capacity of 51 mAh g−1 at 0.1 C rate for 40 cycles which corresponds to a reversible intercalation/de-intercalation of 1.3 sodium ions. The structural deformation has been observed during the charge–discharge process beyond the removal of 1.3 Na+ ions and has been confirmed by in situ PXRD measurements. The present results provide a guideline to improve the performances of the high-voltage Na4Ni3(PO4)2P2O7 material for the next generation sodium-ion batteries." @default.
• W2989689433 created "2019-12-05" @default.
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• W2989689433 date "2019-11-26" @default.
• W2989689433 modified "2023-10-13" @default.
• W2989689433 title "Electrochemical investigations of high-voltage Na4Ni3(PO4)2P2O7 cathode for sodium-ion batteries" @default.
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• W2989689433 doi "https://doi.org/10.1007/s10008-019-04448-6" @default.
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