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- W2989710626 abstract "In the development of two-dimension (2D) materials, constructing orderly layer-by-layered heterostructure has been a formidable challenge for a long time. In this work, a convenient nitriding-pretreatment route has been applied to engineer the C vacancy defects in Ti3C2Tx MXene, which often results in the structural instability. Based on the above defect engineering, the 2D skeleton is maintained in the following Ti3C2Tx oxidation for the formation of TiO2 and carbon layers. Successfully, a “from 2D to 2D” structure and functional transformation is realized and TiO2 nanoplates are in-situ grown between carbon layers, which greatly boost photogenerated carrier’s separation and electron’s transmission. As a result, this TiO2/C superstructure exhibits an efficient photocatalytic ability in water-splitting process under visible light without any cocatalyst (87.2 μmol g−1 h−1, 28.1 times of disordered TiO2/C sample). The defect engineering for MXene provides a new strategy for the highly orderly layer-by-layer superstructure." @default.
- W2989710626 created "2019-12-05" @default.
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- W2989710626 date "2020-01-01" @default.
- W2989710626 modified "2023-10-16" @default.
- W2989710626 title "Orderly layer-by-layered TiO2/carbon superstructures based on MXene’s defect engineeringfor efficient hydrogen evolution" @default.
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- W2989710626 doi "https://doi.org/10.1016/j.apcata.2019.117341" @default.
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