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• W2990160720 abstract "We investigate vapor homogeneous nucleation in a superheated Lennard Jones liquid with computer simulations. Special simulation techniques are required to address this study since the nucleation of a critical vapor bubble --one that has equal chance to grow or shrink-- in a moderately superheated liquid is a rare event. We use the Seeding method, that combines Classical Nucleation Theory with computer simulations of a liquid containing a vapor bubble to provide bubble nucleation rates in a wide temperature range. Seeding has been successfully applied to investigate the nucleation of crystals in supercooled fluids and here we apply it for the fist time --to the best of our knowledge-- to the liquid-to-vapor transition. We find that Seeding provides nucleation rates that are consistent with independent calculations not based on the assumptions of Classical Nucleation Theory. Different criteria to determine the radius of the critical bubble give different rate values. The accuracy of each criterion depends of the degree of superheating. Moreover, Seeding simulations show that the surface tension depends on pressure for a given temperature. Therefore, using Classical Nucleation Theory with the coexistence surface tension does not provide good estimates of the nucleation rate." @default.
• W2990160720 created "2019-12-05" @default.
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• W2990160720 date "2019-11-20" @default.
• W2990160720 modified "2023-10-14" @default.
• W2990160720 title "Seeding approach to bubble nucleation in superheated Lennard-Jones fluids" @default.
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• W2990160720 doi "https://doi.org/10.1103/physreve.100.052609" @default.
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