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• W2990172036 endingPage "108955" @default.
• W2990172036 startingPage "108955" @default.
• W2990172036 abstract "2,4-Dichlorophenol (2,4-DCP) is a hazardous chlorinated organic chemical derived from phenol that exerts serious effects on living organisms. In the present study, SnO2 templated with grapefruit peel carbon as a nanocomposite (SnO2@GPC) was designed via ball-milling, and its mechanism of 2,4-DCP adsorption in aqueous solution was determined. Batch adsorption experiments revealed that the maximum adsorption efficiency of SnO2@GPC occurred at 6.0 pH, 3 mg L−1 initial adsorbate concentration, 2 h contact time, and 293 K temperature. The SnO2@GPC nanocomposite and its non-tin-bearing counterpart, grapefruit derived char (@GPC), showed maximum adsorption capacities (QL) of 45.95 and 22.09 mg g−1 and partition coefficients of 41.77 and 10.83 mg g−1 μM−1, respectively. The adsorption of 2,4-DCP was best described by the Redlich−Peterson model followed by the Langmuir model with high correlation coefficients (R2 ≥ 0.96), and the adsorption kinetic data best fitted the pseudo-second-order model (R2 ≥ 0.98). The thermodynamic parameters indicated that the reaction was spontaneous, exothermic, and involved high affinity between SnO2@GPC and 2,4-DCP. The high desorption efficiency obtained (>80%) demonstrated the recyclability of the adsorbent. The enhanced QL of SnO2@GPC was due to the effective combination of GPC and SnO2. A thin porous layer of GPC on SnO2 nanoparticles provided effective channels, a large surface area, and an abundance of active sites for 2,4-DCP adsorption. Thus, the SnO2@GPC nanocomposite could potentially be used as a low-cost adsorbent to remove 2,4-DCP from water." @default.
• W2990172036 created "2019-12-05" @default.
• W2990172036 creator A5014917742 @default.
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• W2990172036 date "2020-02-01" @default.
• W2990172036 modified "2023-10-16" @default.
• W2990172036 title "Design and characterization of a biomass template/SnO2 nanocomposite for enhanced adsorption of 2,4-dichlorophenol" @default.
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• W2990172036 doi "https://doi.org/10.1016/j.envres.2019.108955" @default.
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• W2990172036 hasPublicationYear "2020" @default.
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