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- W2990196046 abstract "A nanocage coupling effect from a redox RuII -PdII metal-organic cage (MOC-16) is demonstrated for efficient photochemical H2 production by virtue of redox-guest modulation of the photo-induced electron transfer (PET) process. Through coupling with photoredox cycle of MOC-16, tetrathiafulvalene (TTF) guests act as electron relay mediator to improve the overall electron transfer efficiency in the host-guest system in a long-time scale, leading to significant promotion of visible-light driven H2 evolution. By contrast, the presence of larger TTF-derivatives in bulk solution without host-guest interactions results in interference with PET process of MOC-16, leading to inefficient H2 evolution. Such interaction provides an example to understand the interplay between the redox-active nanocage and guest for optimization of redox events and photocatalytic activities in a confined chemical nanoenvironment." @default.
- W2990196046 created "2019-12-05" @default.
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- W2990196046 date "2019-12-17" @default.
- W2990196046 modified "2023-10-14" @default.
- W2990196046 title "The Redox Coupling Effect in a Photocatalytic Ru<sup>II</sup>‐Pd<sup>II</sup> Cage with TTF Guest as Electron Relay Mediator for Visible‐Light Hydrogen‐Evolving Promotion" @default.
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- W2990196046 doi "https://doi.org/10.1002/anie.201913303" @default.
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