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- W2990555903 abstract "Abstract It is believed that porous heterogeneous materials with excellent properties are promising candidates for efficient fixation of diluted and waste CO2. Herein, a family of mesoporous porous ionic copolymers (PIPs) was designed and prepared from the copolymerization of divinylbenzene (DVB) with vinyl-functionalized ionic liquids monomers through free radical copolymerization process. It was demonstrated that the heterogeneous PIP poly(divinylbenzene-1-allyl-tetramethylguanidinium bromide) PDVB-[AlTMG]Br-0.2 showed excellent activities in facile cycloaddition of CO2 into cyclic carbonates without using any external co-catalysts or metal additives. The results of characterizations and quantum mechanical calculations further showed that the specic hierarchical meso-macroporous structure of PDVB-[AlTMG]Br-0.2 offered the strongest binding interaction with SO and besides had a relatively good CO2 affinity, which results to the best cataltic activity for cycloaddition of CO2. Moreover, PDVB-[AlTMG]Br-0.2 exhibited high activities and good reusability in cycloaddition of 15 % diluted CO2 with various epoxides. It is believed that our work would have a great potential in energy-effective fixation of industrial combustion CO2 into high-value organic carbonates." @default.
- W2990555903 created "2019-12-05" @default.
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- W2990555903 date "2020-02-01" @default.
- W2990555903 modified "2023-10-12" @default.
- W2990555903 title "Highly efficient cycloaddition of diluted and waste CO2 into cyclic carbonates catalyzed by porous ionic copolymers" @default.
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- W2990555903 doi "https://doi.org/10.1016/j.jcou.2019.11.003" @default.
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