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- W2990748918 abstract "Catalytic elimination of chlorinated volatile organic compounds (CVOCs) from the industrial sources of emission usually confronted with catalyst deactivation and secondary pollution. As a widely used catalyst in selective catalytic reduction (SCR) of nitric oxides, V2O5-WO3/TiO2 catalysts (denoted as VWT) have been also applied for eliminating the CVOCs, especially those from the municipal solid waste (MSW) incineration. However, the effect of heavy metals on the reaction characteristics of this catalyst is lack of exploration, which has been considered to be a main cause for catalyst deactivation. Herein, we investigated the effect of lead (Pb), a critical heavy meal in the flue gas of MSW incineration, on the catalytic elimination of chlorobenzene (CB) over the VWT catalyst. Variations of catalytic activity, CO2/HCl selectivity and chlorine adsorption/desorption behaviors were evaluated. In particular, the reaction byproducts with and without Pb loadings were qualitatively and quantitatively analyzed. It was noted that the loading of excessive Pb could change the reaction route over the VWT catalyst, leading to low CB oxidation efficiency and CO2 selectivity. However, these Pb spices likely acted as a sink to capture the dissociated Cl that hindered the electrophilic chlorination reaction, and avoided the formation of more toxic polychlorinated byproducts." @default.
- W2990748918 created "2019-12-05" @default.
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- W2990748918 date "2020-04-01" @default.
- W2990748918 modified "2023-10-14" @default.
- W2990748918 title "Elimination of chloroaromatic congeners on a commercial V2O5-WO3/TiO2 catalyst: The effect of heavy metal Pb" @default.
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- W2990748918 doi "https://doi.org/10.1016/j.jhazmat.2019.121705" @default.
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