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• W2991336696 endingPage "118473" @default.
• W2991336696 startingPage "118473" @default.
• W2991336696 abstract "Planar laser-induced fluorescence is employed as noninvasive in situ technique to investigate the oxidation of formaldehyde over platinum. Two-dimensional absolute HCHO concentration distributions over a catalyst-coated plate are visualized in a parallel wall channel. The experimental results are compared with corresponding numerical simulations using ANSYS-Fluent with a detailed surface reaction mechanism. The influence of temperature, Pt-loading and mass flow rate on HCHO profiles are investigated experimentally and numerically in steady state. In the temperature range of 373 – 673 K, the HCHO distribution measured is well predicted by the model. A slow transition from a kinetically controlled regime to a mass transfer limited regime can be observed at 573 K in this study. It is found that the local HCHO concentration in the catalytic channel is governed by a combined effect of chemical kinetics, diffusive mass transfer, and flow field." @default.
• W2991336696 created "2019-12-05" @default.
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• W2991336696 date "2020-05-01" @default.
• W2991336696 modified "2023-10-10" @default.
• W2991336696 title "Investigation of HCHO Catalytic Oxidation over Platinum using Planar Laser-Induced Fluorescence" @default.
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• W2991336696 doi "https://doi.org/10.1016/j.apcatb.2019.118473" @default.
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