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- W2991628841 abstract "Despite many cationic nanomaterials that have been developed for efficient adsorption of anionic pollutants, tailoring a stable shape with denser cations on the surface for advanced removal capability remains challenging. Here, a new strategy is presented for fabricating two-dimensional (2D) cationic laminas and their curvature based on cross-linking of 2D supramolecular networks from hydrogen-bonded trimesic amide derivatives. Owing to the distribution of most cations on the surface, two cationic nanostructures from cross-linking of supramolecular networks show fast sorption kinetics for anionic pollutants. Notably, the removal capacity of the capsule-like curvature adsorbent is more than twice that of lamina adsorbent for sufficient space around cationic sites in hollow aperture. Moreover, the capsule-like adsorbent is triggered to open and spontaneously release the adsorbed pollutants upon the addition of halogen anions, which can be recovered by subsequent dialysis. Strategy of a capsule-like pocket with tunable opening–closing will provide a new insight for storage and adsorption." @default.
- W2991628841 created "2019-12-05" @default.
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- W2991628841 date "2019-11-26" @default.
- W2991628841 modified "2023-10-11" @default.
- W2991628841 title "Two-Dimensional Cationic Networks and Their Spherical Curvature with Tunable Opening–Closing" @default.
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- W2991628841 doi "https://doi.org/10.1021/acs.nanolett.9b04421" @default.
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