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• W2993881418 abstract "H2 permeability of the mixed protonic and electronic conducting membranes can be enhanced by the adjustment of the operating conditions. BaCe0.8Y0.2O3−δ (BCY)–Ce0.8Y0.2O2−δ (YDC)/BCY–Ni hollow fiber membranes were prepared, and their H2 permeation fluxes under a gas atmosphere containing water vapor and CO2 were systematically investigated. The influences of H2 partial pressure in feed stream, steam, or CO2 concentration in sweep gas, sweep gas flow rate, and operating temperature on H2 permeation fluxes were studied. When the sweep side was humidified, the H2 permeation flux of the membrane was increased and reached 1.21 mL cm–2 min–1 at 900 °C. When using 20% CO2–N2 as the sweep gas, H2 permeation flux of the membrane was further increased because of the presence of the reverse water–gas shift (RWGS) reaction, achieving 3.03 mL cm–2 min–1 at 900 °C, one of the highest H2 fluxes ever reported for mixed protonic and electronic conducting membranes. Without adding extra catalyst, the conversion of CO2 reached 42.5% when using 7% CO2–N2 as the sweep gas at 900 °C, indicating that the membrane material itself has a certain catalytic activity for RWGS. In addition to the excellent H2 permeability, the membrane also showed good stability in a H2–CO2-containing atmosphere, highlighting its promising application as the membrane reactor for H2 separation and CO2 transformation." @default.
• W2993881418 created "2019-12-13" @default.
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• W2993881418 date "2019-12-06" @default.
• W2993881418 modified "2023-10-16" @default.
• W2993881418 title "CO₂ and Steam-Assisted H₂ Separation through BaCe_0.8Y_0.2O_3−δ–Ce_0.8Y_0.2O_2−δ Hollow Fiber Membranes" @default.
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• W2993881418 doi "https://doi.org/10.1021/acs.energyfuels.9b02972" @default.
• W2993881418 hasPublicationYear "2019" @default.
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