Matches in SemOpenAlex for { <https://semopenalex.org/work/W2993963917> ?p ?o ?g. }
Showing items 1 to 69 of
69
with 100 items per page.
- W2993963917 endingPage "44" @default.
- W2993963917 startingPage "38" @default.
- W2993963917 abstract "在硅烷偶联剂(3-环氧乙基甲氧基丙基)三甲氧基硅烷(GPTMS)作用下合成了多级孔结构Fe-ZSM-5，采用氨水蒸气对Fe-ZSM-5分子筛进行后处理。利用XRD、SEM、N2吸脱附、UV-vis及NH3-TPD等方法对处理的Fe-ZSM-5进行了表征，并考察了处理后的沸石分子筛催化N2O氧化苯制苯酚的催化性能。结果表明，氨水蒸气相较于水蒸气处理的Fe-ZSM-5分子筛骨架结构和孔结构变化不大，但保留了更多的中强酸酸中心和非骨架活性铁物种，在苯制苯酚反应中表现出更好的催化活性。 Hierarchical Fe-ZSM-5 was synthesized with the aid of 3-glycidoxypropyltrimethoxysilane (GPTMS) and then was modified by the ammonia-steaming post treatment. Various techniques, such as XRD, SEM, N2 adsorption-desorption, UV-vis and NH3-TPD were used to characterize the as-obtained and modified hierarchical Fe-ZSM-5. The direct oxidation of benzene to phenol using N2O as the oxidizing agent was conducted on the ammonia-steaming treated Fe-ZSM-5. The results showed that compared to the steaming treated Fe-ZSM-5 catalysts, ammonia-steaming treated hierarchical Fe-ZSM-5 catalysts preserved more mediate strong acid sites and ex-framework iron active species, thus exhibited a higher catalytic activity in the catalytic oxidation of benzene to phenol with N2O, while the frame structure and pore structure of Fe-ZSM-5 was almost unchange." @default.
- W2993963917 created "2019-12-13" @default.
- W2993963917 creator A5015104874 @default.
- W2993963917 date "2015-01-01" @default.
- W2993963917 modified "2023-09-25" @default.
- W2993963917 title "Direct Oxidation of Benzene to Phenol by N<sub>2</sub>O over Fe-ZSM-5 Zeolites Obtained via Ammonia-Steaming Treatment" @default.
- W2993963917 cites W1978135775 @default.
- W2993963917 cites W1982303619 @default.
- W2993963917 cites W1984227886 @default.
- W2993963917 cites W1985863113 @default.
- W2993963917 cites W2003180136 @default.
- W2993963917 cites W2022307288 @default.
- W2993963917 cites W2052827433 @default.
- W2993963917 cites W2057219172 @default.
- W2993963917 cites W2072388752 @default.
- W2993963917 cites W2083796312 @default.
- W2993963917 cites W2087407801 @default.
- W2993963917 cites W2135809158 @default.
- W2993963917 cites W2142920551 @default.
- W2993963917 cites W2951106791 @default.
- W2993963917 doi "https://doi.org/10.12677/japc.2015.42006" @default.
- W2993963917 hasPublicationYear "2015" @default.
- W2993963917 type Work @default.
- W2993963917 sameAs 2993963917 @default.
- W2993963917 citedByCount "0" @default.
- W2993963917 crossrefType "journal-article" @default.
- W2993963917 hasAuthorship W2993963917A5015104874 @default.
- W2993963917 hasBestOaLocation W29939639171 @default.
- W2993963917 hasConcept C161790260 @default.
- W2993963917 hasConcept C178790620 @default.
- W2993963917 hasConcept C185592680 @default.
- W2993963917 hasConcept C2776382133 @default.
- W2993963917 hasConcept C2777691172 @default.
- W2993963917 hasConcept C2777702071 @default.
- W2993963917 hasConcept C2778077586 @default.
- W2993963917 hasConcept C2778533180 @default.
- W2993963917 hasConcept C2779023244 @default.
- W2993963917 hasConcept C31903555 @default.
- W2993963917 hasConceptScore W2993963917C161790260 @default.
- W2993963917 hasConceptScore W2993963917C178790620 @default.
- W2993963917 hasConceptScore W2993963917C185592680 @default.
- W2993963917 hasConceptScore W2993963917C2776382133 @default.
- W2993963917 hasConceptScore W2993963917C2777691172 @default.
- W2993963917 hasConceptScore W2993963917C2777702071 @default.
- W2993963917 hasConceptScore W2993963917C2778077586 @default.
- W2993963917 hasConceptScore W2993963917C2778533180 @default.
- W2993963917 hasConceptScore W2993963917C2779023244 @default.
- W2993963917 hasConceptScore W2993963917C31903555 @default.
- W2993963917 hasIssue "02" @default.
- W2993963917 hasLocation W29939639171 @default.
- W2993963917 hasOpenAccess W2993963917 @default.
- W2993963917 hasPrimaryLocation W29939639171 @default.
- W2993963917 hasRelatedWork W153939838 @default.
- W2993963917 hasRelatedWork W1969502482 @default.
- W2993963917 hasRelatedWork W1982303619 @default.
- W2993963917 hasRelatedWork W2001872281 @default.
- W2993963917 hasRelatedWork W2014119185 @default.
- W2993963917 hasRelatedWork W2951351940 @default.
- W2993963917 hasRelatedWork W2993963917 @default.
- W2993963917 hasRelatedWork W2472190149 @default.
- W2993963917 hasRelatedWork W2519266192 @default.
- W2993963917 hasRelatedWork W2536607990 @default.
- W2993963917 hasVolume "04" @default.
- W2993963917 isParatext "false" @default.
- W2993963917 isRetracted "false" @default.
- W2993963917 magId "2993963917" @default.
- W2993963917 workType "article" @default.