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• W2993976021 endingPage "135431" @default.
• W2993976021 startingPage "135431" @default.
• W2993976021 abstract "Transition metal phosphides are emerging non-noble metal electrocatalysts for hydrogen evolution reaction (HER) in water splitting. Herein, porous nickel cobalt phosphide nanosheet arrays with hierarchical structure were synthesized on carbon cloth (NiCoxPy-P/CC) as a robust and stable HER electrocatalyst by a facile approach involving electrodeposition and an effective PH3 plasma-assisted phosphorization. Owing to the unique structure with porous nanosheets composed of defect-abundant fine nanocrystals, the as-synthesized NiCoxPy/CC electrocatalyst demonstrates superior catalytic activity for HER to its thermally-phosphorized counterpart. Only at the overpotential as low as 70 (in 0.5 M H2SO4) and 42 mV (in 1 M KOH), the current density of 10 mA/cm2 is achieved for the NiCoxPy/CC, which is among the best reported values for metal phosphide electrocatalysts. Moreover, the catalyst shows satisfying long-term durability up to 24 h in both the acidic and alkaline media. The outstanding HER performance and efficient synthesis strategy for the NiCoxP-P/CC makes it a promising electrocatalyst for hydrogen production." @default.
• W2993976021 created "2019-12-13" @default.
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• W2993976021 date "2020-01-01" @default.
• W2993976021 modified "2023-10-13" @default.
• W2993976021 title "Plasma-assisted synthesis of hierarchical NiCoxPy nanosheets as robust and stable electrocatalyst for hydrogen evolution reaction in both acidic and alkaline media" @default.
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• W2993976021 doi "https://doi.org/10.1016/j.electacta.2019.135431" @default.
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