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- W2995388889 abstract "Large deviation functions contain information on the stability and response of systems driven into nonequilibrium steady states and in such a way are similar to free energies for systems at equilibrium. As with equilibrium free energies, evaluating large deviation functions numerically for all but the simplest systems is difficult because by construction they depend on exponentially rare events. In this first paper of a series, we evaluate different trajectory-based sampling methods capable of computing large deviation functions of time integrated observables within nonequilibrium steady states. We illustrate some convergence criteria and best practices using a number of different models, including a biased Brownian walker, a driven lattice gas, and a model of self-assembly. We show how two popular methods for sampling trajectory ensembles, transition path sampling and diffusion Monte Carlo, suffer from exponentially diverging correlations in trajectory space as a function of the bias parameter when estimating large deviation functions. Improving the efficiencies of these algorithms requires introducing guiding functions for the trajectories." @default.
- W2995388889 created "2019-12-26" @default.
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- W2995388889 date "2018-03-28" @default.
- W2995388889 modified "2023-09-29" @default.
- W2995388889 title "Importance sampling large deviations in nonequilibrium steady states. I" @default.
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- W2995388889 doi "https://doi.org/10.1063/1.5003151" @default.
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