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- W2995484287 abstract "Two-dimensional layered organic-inorganic perovskite hybrids have attracted increasing attention due to their outstanding moisture resistance and promising optoelectronic properties. However, the photovoltaic performance in solar cells is still a huge challenge for two-dimensional perovskite films. With the aim to improve the efficiency of 2D perovskite solar cells, the new (ClC6H4C2H4NH3)2MAn−1PbnI3n+1 perovskite family (abbreviated as (CPEA)2MAn−1PbnI3n+1) are synthesized by a simple one-step hot-casting method in this study. It is found that the variation of n value (n = 3–6) has great influence on the microstructure, grain size, charge mobility, trap density and photovoltaic performance of the 2D (CPEA)2(MA)n−1PbnI3n+1. Due to the best film quality and prolonged carrier lifetime, the (CPEA)2MA4Pb5I16 (n = 5) perovskite solar cell exhibits a highest efficiency of 11.86%, with a Voc of 0.989 V, a Jsc of 19.92 mA/cm2 and FF of 60%, respectively. It is anticipated that our approach to explore new organic spacer cations in 2D perovskites may pave the way for their application with high performance." @default.
- W2995484287 created "2019-12-26" @default.
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- W2995484287 date "2020-01-01" @default.
- W2995484287 modified "2023-10-12" @default.
- W2995484287 title "2D multilayered perovskites based on 4-chlorophenylethylamine for solar cell application" @default.
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- W2995484287 doi "https://doi.org/10.1016/j.solener.2019.12.021" @default.
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