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- W2995970219 abstract "Single-atom catalysts (SACs) have attracted broad interest recently due to their superior catalytic properties. However, a facile fabrication method for the large-scale synthesis of SACs is still in demand. This study reports a mechanochemical approach for the mass production of noble metal SACs. The successful formation of atomically dispersed palladium species on zinc oxide (Pd1/ZnO) was verified by aberration-corrected high-angle annular dark-field scanning transmission electron microscopy and X-ray absorption spectroscopy. Furthermore, our method exhibited little scaling-up effect on the mass production of Pd1/ZnO at ranges of 10–1,000 g, in which the catalyst structure and catalytic performance were retained. Meanwhile, the versatility of this approach was demonstrated by the large-scale fabrication of Rh and Ru SACs, and Pd1/Cu single-atom alloys. Thus, this promising strategy provides the potential for cost-effective mass production of SACs and subsequently may open a window for their industrial application." @default.
- W2995970219 created "2019-12-26" @default.
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- W2995970219 date "2020-01-01" @default.
- W2995970219 modified "2023-10-17" @default.
- W2995970219 title "Mechanochemical Kilogram-Scale Synthesis of Noble Metal Single-Atom Catalysts" @default.
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- W2995970219 doi "https://doi.org/10.1016/j.xcrp.2019.100004" @default.
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