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• W2996586464 endingPage "787" @default.
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• W2996586464 abstract "Quantifying and predicting the solubility of minerals in saline aqueous fluids across wide ranges of pressure, temperature and salinity is critical for interpreting geologic processes. Here, we define a new thermodynamic model for mineral solubility in saline aqueous fluids. The model is based in part on coupling two previous models: one for the solubility of minerals in pure H₂O fluids as function of temperature and fluid density (Dolejš and Manning, 2010), with the additional effects of salinity modeled based in part on Akinfiev and Diamond (2009), with some modifications and additions. Specifically, the new model adopts a modified version of the approach by Akinfiev and Diamond (2009) to incorporate the effect salinity on solvent density, with additional expressions added for the equilibrium constants of reactions involving explicit sodium and/or chloride species. The new generic model is applicable to the solubility of minerals that dissolve as hydrous species, sodium and/or chloride species, and combinations thereof. The model has been calibrated according to experimentally determined solubilities for six common rock-forming minerals – quartz, calcite, corundum, fluorapatite, fluorite, and rutile – in H₂O-NaCl solutions at temperatures up to 1100 °C and pressures up to 20 kbar. Data and trends in experimental measurements are well reproduced by the model, and the accuracy is within experimental uncertainty. In the case of pure H₂O fluids (zero salinity), the model is implicitly equivalent to that of Dolejš and Manning (2010). This thermodynamic model, accounting for dissolution reactions in saline fluids over an extreme range of pressure, temperature and salinity, will allow for robust modeling of reactions and mass transport in natural systems." @default.
• W2996586464 created "2019-12-26" @default.
• W2996586464 creator A5018600577 @default.
• W2996586464 creator A5032535664 @default.
• W2996586464 date "2019-11-01" @default.
• W2996586464 modified "2023-10-12" @default.
• W2996586464 title "A model for the solubility of minerals in saline aqueous fluids in the crust and upper mantle" @default.
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• W2996586464 doi "https://doi.org/10.2475/09.2019.02" @default.
• W2996586464 hasPublicationYear "2019" @default.
• W2996586464 type Work @default.
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