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- W2997123410 abstract "Abstract This study demonstrated a new method for simultaneously improving the interfacial morphology and gas separation properties of mixed matrix membrane by designing a new type of nanocomposite filler (UiO-66-PEI@[bmim][Tf2N]). Nano-sized UiO-66 particle was post-synthetically modified with branched polyethyleneimine (PEI) and then was decorated with ionic liquid. The abundant amino groups in UiO-66-PEI improve the gas separation properties of the MMM due to the affinity between PEI and CO2. The ionic liquid acts as a lubricant agent, which is coated on the crystal surface improves the interface morphology of the MMM. Compared to pristine 6FO and MOF/6FO membrane, MOF@IL/6FO membrane has higher gas separation performance. Characterization and gas separation results indicated the UiO-66-PEI@ILs particles were homogeneous dispersed in 6FDA-ODA and promoted CO2 transport by reversible reaction with amine groups. Consequently, the membrane sample containing 15 wt% loading of the UiO-66-PEI@[bmim][Tf2N] filler displayed an optimum CO2/CH4 selectivity of 59.99 for CO2 and CH4 mixture gas." @default.
- W2997123410 created "2020-01-10" @default.
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- W2997123410 date "2020-05-01" @default.
- W2997123410 modified "2023-10-16" @default.
- W2997123410 title "Improved CO2 separation performance and interfacial affinity of mixed matrix membrane by incorporating UiO-66-PEI@[bmim][Tf2N] particles" @default.
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- W2997123410 doi "https://doi.org/10.1016/j.seppur.2020.116519" @default.
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