Matches in SemOpenAlex for { <https://semopenalex.org/work/W2997260047> ?p ?o ?g. }
- W2997260047 endingPage "1470" @default.
- W2997260047 startingPage "1461" @default.
- W2997260047 abstract "Cerium(IV)-driven water oxidation catalysis mediated by a mononuclear ruthenium(III) complex, [Ru(L)(pic)3] (H3L = 2,2′-iminodibenzoic acid, pic = 4-methylpyridine), has been demonstrated in this work. The mechanistic details of water oxidation have been investigated by the combined use of spectroscopy, electrochemistry, kinetic analysis, and computational studies. It was found that water oxidation proceeds via formal high-valent RuVII species. The capability of accessing such a high-valent state is derived from the non-innocent behavior of the anionic tridentate ligand frame which helps in accumulation of oxidative equivalents in cooperation with metal center. This metal–ligand cooperation facilitates the multi-electron-transfer reaction such as water oxidation. Kinetic analysis suggests water oxidation at a single site of Ru where O–O bond formation occurs via radical–radical coupling pathway between the oxygen atom of ruthenium-oxo species and the oxygen atom of the hydroxocerium(IV) ion." @default.
- W2997260047 created "2020-01-10" @default.
- W2997260047 creator A5007860158 @default.
- W2997260047 creator A5018509718 @default.
- W2997260047 creator A5021369452 @default.
- W2997260047 creator A5057674766 @default.
- W2997260047 creator A5085643455 @default.
- W2997260047 date "2019-12-26" @default.
- W2997260047 modified "2023-10-01" @default.
- W2997260047 title "Mononuclear Ruthenium-Based Water Oxidation Catalyst Supported by Anionic, Redox-Non-Innocent Ligand: Heterometallic O–O Bond Formation via Radical Coupling Pathway" @default.
- W2997260047 cites W1874296098 @default.
- W2997260047 cites W1967895364 @default.
- W2997260047 cites W1977892176 @default.
- W2997260047 cites W1983293320 @default.
- W2997260047 cites W1985067760 @default.
- W2997260047 cites W1988324461 @default.
- W2997260047 cites W2012046411 @default.
- W2997260047 cites W2030938880 @default.
- W2997260047 cites W2048082715 @default.
- W2997260047 cites W2053834882 @default.
- W2997260047 cites W2055663482 @default.
- W2997260047 cites W2056450153 @default.
- W2997260047 cites W2060663357 @default.
- W2997260047 cites W2083323519 @default.
- W2997260047 cites W2085256740 @default.
- W2997260047 cites W2091758842 @default.
- W2997260047 cites W2107285918 @default.
- W2997260047 cites W2118082954 @default.
- W2997260047 cites W2120236380 @default.
- W2997260047 cites W2121832548 @default.
- W2997260047 cites W2171093931 @default.
- W2997260047 cites W2239220623 @default.
- W2997260047 cites W2269306364 @default.
- W2997260047 cites W2314821493 @default.
- W2997260047 cites W2322210206 @default.
- W2997260047 cites W2331224612 @default.
- W2997260047 cites W2334491264 @default.
- W2997260047 cites W2469545046 @default.
- W2997260047 cites W2494300389 @default.
- W2997260047 cites W2552423250 @default.
- W2997260047 cites W2561587734 @default.
- W2997260047 cites W2594171890 @default.
- W2997260047 cites W2595697336 @default.
- W2997260047 cites W2753178629 @default.
- W2997260047 cites W2794687760 @default.
- W2997260047 cites W2888495858 @default.
- W2997260047 cites W2898346398 @default.
- W2997260047 cites W2941990132 @default.
- W2997260047 cites W4238850712 @default.
- W2997260047 cites W4376595665 @default.
- W2997260047 doi "https://doi.org/10.1021/acs.inorgchem.9b03258" @default.
- W2997260047 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/31877037" @default.
- W2997260047 hasPublicationYear "2019" @default.
- W2997260047 type Work @default.
- W2997260047 sameAs 2997260047 @default.
- W2997260047 citedByCount "16" @default.
- W2997260047 countsByYear W29972600472021 @default.
- W2997260047 countsByYear W29972600472022 @default.
- W2997260047 countsByYear W29972600472023 @default.
- W2997260047 crossrefType "journal-article" @default.
- W2997260047 hasAuthorship W2997260047A5007860158 @default.
- W2997260047 hasAuthorship W2997260047A5018509718 @default.
- W2997260047 hasAuthorship W2997260047A5021369452 @default.
- W2997260047 hasAuthorship W2997260047A5057674766 @default.
- W2997260047 hasAuthorship W2997260047A5085643455 @default.
- W2997260047 hasConcept C116569031 @default.
- W2997260047 hasConcept C123669783 @default.
- W2997260047 hasConcept C161790260 @default.
- W2997260047 hasConcept C170493617 @default.
- W2997260047 hasConcept C178790620 @default.
- W2997260047 hasConcept C179104552 @default.
- W2997260047 hasConcept C185592680 @default.
- W2997260047 hasConcept C2778591166 @default.
- W2997260047 hasConcept C523597863 @default.
- W2997260047 hasConcept C544153396 @default.
- W2997260047 hasConcept C55493867 @default.
- W2997260047 hasConcept C555196967 @default.
- W2997260047 hasConcept C55904794 @default.
- W2997260047 hasConcept C75473681 @default.
- W2997260047 hasConcept C83155894 @default.
- W2997260047 hasConcept C89477785 @default.
- W2997260047 hasConceptScore W2997260047C116569031 @default.
- W2997260047 hasConceptScore W2997260047C123669783 @default.
- W2997260047 hasConceptScore W2997260047C161790260 @default.
- W2997260047 hasConceptScore W2997260047C170493617 @default.
- W2997260047 hasConceptScore W2997260047C178790620 @default.
- W2997260047 hasConceptScore W2997260047C179104552 @default.
- W2997260047 hasConceptScore W2997260047C185592680 @default.
- W2997260047 hasConceptScore W2997260047C2778591166 @default.
- W2997260047 hasConceptScore W2997260047C523597863 @default.
- W2997260047 hasConceptScore W2997260047C544153396 @default.
- W2997260047 hasConceptScore W2997260047C55493867 @default.
- W2997260047 hasConceptScore W2997260047C555196967 @default.
- W2997260047 hasConceptScore W2997260047C55904794 @default.
- W2997260047 hasConceptScore W2997260047C75473681 @default.
- W2997260047 hasConceptScore W2997260047C83155894 @default.
- W2997260047 hasConceptScore W2997260047C89477785 @default.
- W2997260047 hasFunder F4320320719 @default.