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• W2997802871 abstract "A new metal-, oxidant-, and solvent-free ecofriendly domino method has been established for modular synthesis of a diverse range of medicinally promising hydroxyarylated unsymmetrical pyridines in good to high chemical yields with an excellent regioselectivity. This domino process involves a range of N-sulfonyl ketimines as C,N-binucleophiles, enolizable ketones, and aromatic/heteroaromatic aldehydes using ammonium acetate as an ideal promoter under neat conditions, which creates two new C–C bonds and one C–N bond. Notably, the neutral reaction conditions are mild enough to tolerate a range of functionalities and cover a variety of substrates, thus bestowing a powerful avenue to access tri- and tetrasubstituted pyridines including carbo- and heterocyclic fused ones. Interestingly, a practical, scalable, and high-yielding synthesis of pyridylphenol derivatives was successfully accomplished by our unique method." @default.
• W2997802871 created "2020-01-10" @default.
• W2997802871 creator A5001546272 @default.
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• W2997802871 creator A5042212121 @default.
• W2997802871 creator A5049807954 @default.
• W2997802871 creator A5055421585 @default.
• W2997802871 date "2019-12-25" @default.
• W2997802871 modified "2023-10-14" @default.
• W2997802871 title "NH₄OAc-Promoted Domino Route to Hydroxyarylated Unsymmetrical Pyridines under Neat Conditions" @default.
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• W2997802871 doi "https://doi.org/10.1021/acs.joc.9b02896" @default.
• W2997802871 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/31875454" @default.
• W2997802871 hasPublicationYear "2019" @default.
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