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- W2997987908 abstract "Abstract. Recent studies have suggested that the ice nucleating ability of some types of pollen is derived from non-proteinaceous macromolecules. These macromolecules may become dispersed by the rupturing of the pollen sac during wetting and drying cycles in the atmosphere. If true, this mechanism might prove to be a significant source of ice nuclei (IN) concentrations when pollen are present. Here we test this hypothesis by measuring ambient IN concentrations from the beginning to the end of the 2013 pollen season in Raleigh, North Carolina, USA. Air samples were collected using a swirling aerosol collector twice per week and the solutions were analysed for ice nuclei activity using a droplet freezing assay. Rainwater samples were collected at the peak of the pollen season and analysed with the drop freezing assay to compare the potentially enhanced IN concentrations measured near the ground with IN concentrations found aloft. Ambient ice nuclei spectra, defined as the number of ice nuclei per volume of air as a function of temperature, are inferred from the aerosol collector solutions. No general trend was observed between ambient pollen counts and observed IN concentrations, suggesting that ice nuclei multiplication via pollen sac rupturing and subsequent release of macromolecules was not prevalent for the pollen types and meteorological conditions typically encountered in the Southeastern US. A serendipitously sampled collection after a downpour provided evidence for a rain-induced IN burst with an observed IN concentration of approximately 30 per litre, a 30-fold increase over background concentrations at −20 °C. The onset temperature of freezing for these particles was approximately −12 °C, suggesting that the ice nucleating particles were biological in origin. The magnitude of the IN burst was significantly larger than previously observed, providing additional evidence to merit further investigation of a self-regulated feedback cycle between the atmosphere and biosphere via the release of cloud forming particles in rain forest environments." @default.
- W2997987908 created "2020-01-10" @default.
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- W2997987908 date "2013-12-04" @default.
- W2997987908 modified "2023-09-23" @default.
- W2997987908 title "Contribution of pollen to atmospheric ice nuclei concentrations" @default.
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- W2997987908 doi "https://doi.org/10.5194/acpd-13-31673-2013" @default.
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