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- W2998285654 abstract "Abstract Photocatalysts can produce active species in the heterogeneous photocatalytic ozonation (HPO) process, which can efficiently degrade and mineralize organic pollutants. In this study, pristine ZnS and metal-doped (Cu, Ag, Bi, Ga, In) ZnS were synthesized by microwave method. The degradation rate of 4-chlorophenol (4-CP) in HPO process is ranked as Cu/ZnS > Bi/ZnS > Ag/ZnS > In/ZnS > Ga/ZnS > ZnS, which is attributed to the following reasons: (1) the schottky junction formed between ZnS and doped metal can effectively capture electrons as an electron trap, thus inhibiting the recombination of electron-hole pairs; (2) narrow bandgap of Cu/ZnS can enhance electron transport; (3) the valence bands of Ag/ZnS, Bi/ZnS, Ga/ZnS and In/ZnS were more positive than that of pristine ZnS to enhance the oxidization ability of holes. The experimental results showed that the optimal water-intake ozone dose optimal influent ozone dosage was 32 mg/l·min−1 under the optimal initial solution pH of 7. In addition, the possible mechanism of HPO process was proposed and clarified. We believe that metal-doped ZnS has a promising potential to be the photocatalyst for the degradation of organic pollutants." @default.
- W2998285654 created "2020-01-10" @default.
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- W2998285654 date "2020-04-01" @default.
- W2998285654 modified "2023-10-16" @default.
- W2998285654 title "Microwave synthesis of metal-doped ZnS photocatalysts and applications on degrading 4-chlorophenol using heterogeneous photocatalytic ozonation process" @default.
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- W2998285654 doi "https://doi.org/10.1016/j.seppur.2019.116469" @default.
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